Detection of plutonium isotopes at lowest quantities using in-source resonance ionization mass spectrometry
- Publication type:
- Journal article
- Metadata:
-
- Autoren
- S Raeder
- A Hakimi
- N Stoebener
- N Trautmann
- K Wendt
- Autoren-URL
- https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=fis-test-1&SrcAuth=WosAPI&KeyUT=WOS:000310083900008&DestLinkType=FullRecord&DestApp=WOS_CPL
- DOI
- 10.1007/s00216-012-6238-6
- eISSN
- 1618-2650
- Externe Identifier
- Clarivate Analytics Document Solution ID: 024BY
- PubMed Identifier: 22865006
- ISSN
- 1618-2642
- Ausgabe der Veröffentlichung
- 8
- Zeitschrift
- ANALYTICAL AND BIOANALYTICAL CHEMISTRY
- Schlüsselwörter
- Resonance ionization mass spectrometry
- In-source RIMS
- Plutonium
- Isotope ratios
- Paginierung
- 2163 - 2172
- Datum der Veröffentlichung
- 2012
- Status
- Published
- Titel
- Detection of plutonium isotopes at lowest quantities using in-source resonance ionization mass spectrometry
- Sub types
- Article
- Ausgabe der Zeitschrift
- 404
Data source: Web of Science (Lite)
- Other metadata sources:
-
- Autoren
- S Raeder
- A Hakimi
- N Stöbener
- N Trautmann
- K Wendt
- DOI
- 10.1007/s00216-012-6238-6
- eISSN
- 1618-2650
- ISSN
- 1618-2642
- Ausgabe der Veröffentlichung
- 8
- Zeitschrift
- Analytical and Bioanalytical Chemistry
- Sprache
- en
- Online publication date
- 2012
- Paginierung
- 2163 - 2172
- Datum der Veröffentlichung
- 2012
- Status
- Published
- Herausgeber
- Springer Science and Business Media LLC
- Herausgeber URL
- http://dx.doi.org/10.1007/s00216-012-6238-6
- Datum der Datenerfassung
- 2019
- Titel
- Detection of plutonium isotopes at lowest quantities using in-source resonance ionization mass spectrometry
- Ausgabe der Zeitschrift
- 404
Data source: Crossref
- Abstract
- The in-source resonance ionization mass spectrometry technique was applied for quantification of ultratrace amounts of plutonium isotopes as a proof of principle study. In addition to an overall detection limit of 10(4) to 10(5) atoms, this method enables the unambiguous identification and individual quantification of the plutonium isotopes (238)Pu and (241)Pu which are of relevance for dating of radiogenic samples. Due to the element-selective ionization process, these isotopes can be measured even under a high surplus of isobaric contaminations from (238)U or (241)Am, which considerably simplifies chemical preparation. The technique was developed, tested, and characterized on a variety of synthetic and calibration samples and is presently applied to analyze environmental samples.
- Addresses
- Institut für Physik, Johannes Gutenberg-Universität Mainz, Mainz, Germany. raeder@triumf.ca
- Autoren
- S Raeder
- A Hakimi
- N Stöbener
- N Trautmann
- K Wendt
- DOI
- 10.1007/s00216-012-6238-6
- eISSN
- 1618-2650
- Externe Identifier
- PubMed Identifier: 22865006
- Open access
- false
- ISSN
- 1618-2642
- Ausgabe der Veröffentlichung
- 8
- Zeitschrift
- Analytical and bioanalytical chemistry
- Schlüsselwörter
- Plutonium
- Isotopes
- Mass Spectrometry
- Limit of Detection
- Sprache
- eng
- Medium
- Print-Electronic
- Online publication date
- 2012
- Paginierung
- 2163 - 2172
- Datum der Veröffentlichung
- 2012
- Status
- Published
- Datum der Datenerfassung
- 2012
- Titel
- Detection of plutonium isotopes at lowest quantities using in-source resonance ionization mass spectrometry.
- Sub types
- Research Support, Non-U.S. Gov't
- Journal Article
- Ausgabe der Zeitschrift
- 404
Data source: Europe PubMed Central
- Abstract
- The in-source resonance ionization mass spectrometry technique was applied for quantification of ultratrace amounts of plutonium isotopes as a proof of principle study. In addition to an overall detection limit of 10(4) to 10(5) atoms, this method enables the unambiguous identification and individual quantification of the plutonium isotopes (238)Pu and (241)Pu which are of relevance for dating of radiogenic samples. Due to the element-selective ionization process, these isotopes can be measured even under a high surplus of isobaric contaminations from (238)U or (241)Am, which considerably simplifies chemical preparation. The technique was developed, tested, and characterized on a variety of synthetic and calibration samples and is presently applied to analyze environmental samples.
- Date of acceptance
- 2012
- Autoren
- S Raeder
- A Hakimi
- N Stöbener
- N Trautmann
- K Wendt
- Autoren-URL
- https://www.ncbi.nlm.nih.gov/pubmed/22865006
- DOI
- 10.1007/s00216-012-6238-6
- eISSN
- 1618-2650
- Ausgabe der Veröffentlichung
- 8
- Zeitschrift
- Anal Bioanal Chem
- Schlüsselwörter
- Isotopes
- Limit of Detection
- Mass Spectrometry
- Plutonium
- Sprache
- eng
- Country
- Germany
- Paginierung
- 2163 - 2172
- Datum der Veröffentlichung
- 2012
- Status
- Published
- Datum, an dem der Datensatz öffentlich gemacht wurde
- 2013
- Titel
- Detection of plutonium isotopes at lowest quantities using in-source resonance ionization mass spectrometry.
- Sub types
- Journal Article
- Research Support, Non-U.S. Gov't
- Ausgabe der Zeitschrift
- 404
Data source: PubMed
- Beziehungen:
- Property of