Manipulation of charge transfer and transport in plasmonic-ferroelectric hybrids for photoelectrochemical applications
- Publication type:
- Journal article
- Metadata:
-
- Autoren
- Zhijie Wang
- Dawei Cao
- Liaoyong Wen
- Rui Xu
- Manuel Obergfell
- Yan Mi
- Zhibing Zhan
- Nasori Nasori
- Jure Demsar
- Yong Lei
- Autoren-URL
- https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=fis-test-1&SrcAuth=WosAPI&KeyUT=WOS:000369019000002&DestLinkType=FullRecord&DestApp=WOS_CPL
- DOI
- 10.1038/ncomms10348
- Externe Identifier
- Clarivate Analytics Document Solution ID: DC2AG
- PubMed Identifier: 26753764
- ISSN
- 2041-1723
- Zeitschrift
- NATURE COMMUNICATIONS
- Artikelnummer
- ARTN 10348
- Datum der Veröffentlichung
- 2016
- Status
- Published
- Titel
- Manipulation of charge transfer and transport in plasmonic-ferroelectric hybrids for photoelectrochemical applications
- Sub types
- Article
- Ausgabe der Zeitschrift
- 7
Data source: Web of Science (Lite)
- Other metadata sources:
-
- Abstract
- <jats:title>Abstract</jats:title><jats:p>Utilizing plasmonic nanostructures for efficient and flexible conversion of solar energy into electricity or fuel presents a new paradigm in photovoltaics and photoelectrochemistry research. In a conventional photoelectrochemical cell, consisting of a plasmonic structure in contact with a semiconductor, the type of photoelectrochemical reaction is determined by the band bending at the semiconductor/electrolyte interface. The nature of the reaction is thus hard to tune. Here instead of using a semiconductor, we employed a ferroelectric material, Pb(Zr,Ti)O<jats:sub>3</jats:sub> (PZT). By depositing gold nanoparticle arrays and PZT films on ITO substrates, and studying the photocurrent as well as the femtosecond transient absorbance in different configurations, we demonstrate an effective charge transfer between the nanoparticle array and PZT. Most importantly, we show that the photocurrent can be tuned by nearly an order of magnitude when changing the ferroelectric polarization in PZT, demonstrating a versatile and tunable system for energy harvesting.</jats:p>
- Autoren
- Zhijie Wang
- Dawei Cao
- Liaoyong Wen
- Rui Xu
- Manuel Obergfell
- Yan Mi
- Zhibing Zhan
- Nasori Nasori
- Jure Demsar
- Yong Lei
- DOI
- 10.1038/ncomms10348
- eISSN
- 2041-1723
- Ausgabe der Veröffentlichung
- 1
- Zeitschrift
- Nature Communications
- Sprache
- en
- Artikelnummer
- 10348
- Online publication date
- 2016
- Status
- Published online
- Herausgeber
- Springer Science and Business Media LLC
- Herausgeber URL
- http://dx.doi.org/10.1038/ncomms10348
- Datum der Datenerfassung
- 2023
- Titel
- Manipulation of charge transfer and transport in plasmonic-ferroelectric hybrids for photoelectrochemical applications
- Ausgabe der Zeitschrift
- 7
Data source: Crossref
- Abstract
- Utilizing plasmonic nanostructures for efficient and flexible conversion of solar energy into electricity or fuel presents a new paradigm in photovoltaics and photoelectrochemistry research. In a conventional photoelectrochemical cell, consisting of a plasmonic structure in contact with a semiconductor, the type of photoelectrochemical reaction is determined by the band bending at the semiconductor/electrolyte interface. The nature of the reaction is thus hard to tune. Here instead of using a semiconductor, we employed a ferroelectric material, Pb(Zr,Ti)O3 (PZT). By depositing gold nanoparticle arrays and PZT films on ITO substrates, and studying the photocurrent as well as the femtosecond transient absorbance in different configurations, we demonstrate an effective charge transfer between the nanoparticle array and PZT. Most importantly, we show that the photocurrent can be tuned by nearly an order of magnitude when changing the ferroelectric polarization in PZT, demonstrating a versatile and tunable system for energy harvesting.
- Addresses
- Institut für Physik &IMN MacroNano (ZIK), Technische Universität Ilmenau, 98693 Ilmenau, Germany.
- Autoren
- Zhijie Wang
- Dawei Cao
- Liaoyong Wen
- Rui Xu
- Manuel Obergfell
- Yan Mi
- Zhibing Zhan
- Nasori Nasori
- Jure Demsar
- Yong Lei
- DOI
- 10.1038/ncomms10348
- eISSN
- 2041-1723
- Externe Identifier
- PubMed Identifier: 26753764
- PubMed Central ID: PMC4729958
- Funding acknowledgements
- European Research Council: 240144
- Open access
- true
- ISSN
- 2041-1723
- Zeitschrift
- Nature communications
- Sprache
- eng
- Medium
- Electronic
- Online publication date
- 2016
- Open access status
- Open Access
- Paginierung
- 10348
- Datum der Veröffentlichung
- 2016
- Status
- Published
- Publisher licence
- CC BY
- Datum der Datenerfassung
- 2016
- Titel
- Manipulation of charge transfer and transport in plasmonic-ferroelectric hybrids for photoelectrochemical applications.
- Sub types
- Research Support, Non-U.S. Gov't
- research-article
- Journal Article
- Ausgabe der Zeitschrift
- 7
Files
https://www.nature.com/articles/ncomms10348.pdf https://europepmc.org/articles/PMC4729958?pdf=render
Data source: Europe PubMed Central
- Abstract
- Utilizing plasmonic nanostructures for efficient and flexible conversion of solar energy into electricity or fuel presents a new paradigm in photovoltaics and photoelectrochemistry research. In a conventional photoelectrochemical cell, consisting of a plasmonic structure in contact with a semiconductor, the type of photoelectrochemical reaction is determined by the band bending at the semiconductor/electrolyte interface. The nature of the reaction is thus hard to tune. Here instead of using a semiconductor, we employed a ferroelectric material, Pb(Zr,Ti)O3 (PZT). By depositing gold nanoparticle arrays and PZT films on ITO substrates, and studying the photocurrent as well as the femtosecond transient absorbance in different configurations, we demonstrate an effective charge transfer between the nanoparticle array and PZT. Most importantly, we show that the photocurrent can be tuned by nearly an order of magnitude when changing the ferroelectric polarization in PZT, demonstrating a versatile and tunable system for energy harvesting.
- Date of acceptance
- 2015
- Autoren
- Zhijie Wang
- Dawei Cao
- Liaoyong Wen
- Rui Xu
- Manuel Obergfell
- Yan Mi
- Zhibing Zhan
- Nasori Nasori
- Jure Demsar
- Yong Lei
- Autoren-URL
- https://www.ncbi.nlm.nih.gov/pubmed/26753764
- DOI
- 10.1038/ncomms10348
- eISSN
- 2041-1723
- Externe Identifier
- PubMed Central ID: PMC4729958
- Zeitschrift
- Nat Commun
- Sprache
- eng
- Country
- England
- Paginierung
- 10348
- PII
- ncomms10348
- Datum der Veröffentlichung
- 2016
- Status
- Published online
- Datum, an dem der Datensatz öffentlich gemacht wurde
- 2016
- Titel
- Manipulation of charge transfer and transport in plasmonic-ferroelectric hybrids for photoelectrochemical applications.
- Sub types
- Journal Article
- Research Support, Non-U.S. Gov't
- Ausgabe der Zeitschrift
- 7
Data source: PubMed
- Beziehungen:
- Property of