Impact of sample history and solvent effects on pathway control in the supramolecular polymerisation of Au(i)-metallopeptide amphiphiles
- Publikationstyp:
- Zeitschriftenaufsatz
- Metadaten:
-
- Autoren
- Marius Thomas
- Vanessa Lewe
- Jonas Koelsch
- Moritz Urschbach
- Jessica Erlenbusch
- Oliver Sven Stach
- Pol Besenius
- Autoren-URL
- https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=fis-test-1&SrcAuth=WosAPI&KeyUT=WOS:000963794000001&DestLinkType=FullRecord&DestApp=WOS_CPL
- DOI
- 10.1039/d3py00053b
- eISSN
- 1759-9962
- Externe Identifier
- Clarivate Analytics Document Solution ID: D9YY7
- PubMed Identifier: 37124957
- ISSN
- 1759-9954
- Ausgabe der Veröffentlichung
- 16
- Zeitschrift
- POLYMER CHEMISTRY
- Paginierung
- 1888 - 1892
- Datum der Veröffentlichung
- 2023
- Status
- Published
- Titel
- Impact of sample history and solvent effects on pathway control in the supramolecular polymerisation of Au(i)-metallopeptide amphiphiles
- Sub types
- Article
- Ausgabe der Zeitschrift
- 14
Datenquelle: Web of Science (Lite)
- Andere Metadatenquellen:
-
- Abstract
- <jats:p>We investigate the kinetics of the supramolecular polymerisation of an Au(<jats:sc>i</jats:sc>)-metallopeptide amphiphile that assembles into exceptionally long and rigid nanofibers.</jats:p>
- Autoren
- Marius Thomas
- Vanessa Lewe
- Jonas Kölsch
- Moritz Urschbach
- Jessica Erlenbusch
- Oliver Sven Stach
- Pol Besenius
- DOI
- 10.1039/d3py00053b
- eISSN
- 1759-9962
- ISSN
- 1759-9954
- Ausgabe der Veröffentlichung
- 16
- Zeitschrift
- Polymer Chemistry
- Sprache
- en
- Online publication date
- 2023
- Paginierung
- 1888 - 1892
- Status
- Published online
- Herausgeber
- Royal Society of Chemistry (RSC)
- Herausgeber URL
- http://dx.doi.org/10.1039/d3py00053b
- Datum der Datenerfassung
- 2024
- Titel
- Impact of sample history and solvent effects on pathway control in the supramolecular polymerisation of Au(<scp>i</scp>)-metallopeptide amphiphiles
- Ausgabe der Zeitschrift
- 14
Datenquelle: Crossref
- Abstract
- We investigate the kinetics of the supramolecular polymerisation of an Au(i)-metallopeptide amphiphile that assembles into exceptionally long and rigid nanofibers. We developed a precise preparation protocol to measure the concentration dependent assembly kinetics which elucidated a nucleation-elongation dominated supramolecular polymerisation process. We show striking differences in the assembly behavior and morphology in aqueous media, even at organic solvent contents as low as 1 vol%, compared to pure buffer.
- Addresses
- Department of Chemistry, Johannes Gutenberg-University Mainz Duesbergweg 10-14 D-55128 Mainz Germany besenius@uni-mainz.de.
- Autoren
- Marius Thomas
- Vanessa Lewe
- Jonas Kölsch
- Moritz Urschbach
- Jessica Erlenbusch
- Oliver Sven Stach
- Pol Besenius
- DOI
- 10.1039/d3py00053b
- eISSN
- 1759-9962
- Externe Identifier
- PubMed Identifier: 37124957
- PubMed Central ID: PMC10127225
- Funding acknowledgements
- Deutsche Forschungsgemeinschaft: Research Training Group RTG 2516 (Grant No. 405552959)
- Studienstiftung des Deutschen Volkes: PhD Scholarship
- European Research Council: 819856
- Deutsche Forschungsgemeinschaft: DFG Excellence Initiative by the Graduate School MAINZ (GSC 266)
- European Research Council: ERC CoG SUPRAVACC - 819856
- Open access
- true
- ISSN
- 1759-9954
- Ausgabe der Veröffentlichung
- 16
- Zeitschrift
- Polymer chemistry
- Sprache
- eng
- Medium
- Electronic-eCollection
- Online publication date
- 2023
- Open access status
- Open Access
- Paginierung
- 1888 - 1892
- Datum der Veröffentlichung
- 2023
- Status
- Published
- Publisher licence
- CC BY
- Datum der Datenerfassung
- 2023
- Titel
- Impact of sample history and solvent effects on pathway control in the supramolecular polymerisation of Au(i)-metallopeptide amphiphiles.
- Sub types
- brief-report
- Journal Article
- Ausgabe der Zeitschrift
- 14
Datenquelle: Europe PubMed Central
- Abstract
- We investigate the kinetics of the supramolecular polymerisation of an Au(i)-metallopeptide amphiphile that assembles into exceptionally long and rigid nanofibers. We developed a precise preparation protocol to measure the concentration dependent assembly kinetics which elucidated a nucleation-elongation dominated supramolecular polymerisation process. We show striking differences in the assembly behavior and morphology in aqueous media, even at organic solvent contents as low as 1 vol%, compared to pure buffer.
- Date of acceptance
- 2023
- Autoren
- Marius Thomas
- Vanessa Lewe
- Jonas Kölsch
- Moritz Urschbach
- Jessica Erlenbusch
- Oliver Sven Stach
- Pol Besenius
- Autoren-URL
- https://www.ncbi.nlm.nih.gov/pubmed/37124957
- DOI
- 10.1039/d3py00053b
- Externe Identifier
- PubMed Central ID: PMC10127225
- ISSN
- 1759-9954
- Ausgabe der Veröffentlichung
- 16
- Zeitschrift
- Polym Chem
- Sprache
- eng
- Country
- England
- Paginierung
- 1888 - 1892
- PII
- d3py00053b
- Datum der Veröffentlichung
- 2023
- Status
- Published online
- Titel
- Impact of sample history and solvent effects on pathway control in the supramolecular polymerisation of Au(i)-metallopeptide amphiphiles.
- Sub types
- Journal Article
- Ausgabe der Zeitschrift
- 14
Datenquelle: PubMed
- Beziehungen:
-