Detection of nanoscale electron spin resonance spectra demonstrated using nitrogen-vacancy centre probes in diamond
- Publikationstyp:
- Zeitschriftenaufsatz
- Metadaten:
-
- Autoren
- LT Hall
- P Kehayias
- DA Simpson
- A Jarmola
- A Stacey
- D Budker
- LCL Hollenberg
- Autoren-URL
- https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=fis-test-1&SrcAuth=WosAPI&KeyUT=WOS:000369019900001&DestLinkType=FullRecord&DestApp=WOS_CPL
- DOI
- 10.1038/ncomms10211
- Externe Identifier
- Clarivate Analytics Document Solution ID: DC2AP
- PubMed Identifier: 26728001
- ISSN
- 2041-1723
- Zeitschrift
- NATURE COMMUNICATIONS
- Artikelnummer
- ARTN 10211
- Datum der Veröffentlichung
- 2016
- Status
- Published
- Titel
- Detection of nanoscale electron spin resonance spectra demonstrated using nitrogen-vacancy centre probes in diamond
- Sub types
- Article
- Ausgabe der Zeitschrift
- 7
Datenquelle: Web of Science (Lite)
- Andere Metadatenquellen:
-
- Abstract
- <jats:title>Abstract</jats:title><jats:p>Electron spin resonance (ESR) describes a suite of techniques for characterizing electronic systems with applications in physics, chemistry, and biology. However, the requirement for large electron spin ensembles in conventional ESR techniques limits their spatial resolution. Here we present a method for measuring ESR spectra of nanoscale electronic environments by measuring the longitudinal relaxation time of a single-spin probe as it is systematically tuned into resonance with the target electronic system. As a proof of concept, we extracted the spectral distribution for the P1 electronic spin bath in diamond by using an ensemble of nitrogen-vacancy centres, and demonstrated excellent agreement with theoretical expectations. As the response of each nitrogen-vacancy spin in this experiment is dominated by a single P1 spin at a mean distance of 2.7 nm, the application of this technique to the single nitrogen-vacancy case will enable nanoscale ESR spectroscopy of atomic and molecular spin systems.</jats:p>
- Autoren
- LT Hall
- P Kehayias
- DA Simpson
- A Jarmola
- A Stacey
- D Budker
- LCL Hollenberg
- DOI
- 10.1038/ncomms10211
- eISSN
- 2041-1723
- Ausgabe der Veröffentlichung
- 1
- Zeitschrift
- Nature Communications
- Sprache
- en
- Artikelnummer
- 10211
- Online publication date
- 2016
- Status
- Published online
- Herausgeber
- Springer Science and Business Media LLC
- Herausgeber URL
- http://dx.doi.org/10.1038/ncomms10211
- Datum der Datenerfassung
- 2023
- Titel
- Detection of nanoscale electron spin resonance spectra demonstrated using nitrogen-vacancy centre probes in diamond
- Ausgabe der Zeitschrift
- 7
Datenquelle: Crossref
- Abstract
- Electron spin resonance (ESR) describes a suite of techniques for characterizing electronic systems with applications in physics, chemistry, and biology. However, the requirement for large electron spin ensembles in conventional ESR techniques limits their spatial resolution. Here we present a method for measuring ESR spectra of nanoscale electronic environments by measuring the longitudinal relaxation time of a single-spin probe as it is systematically tuned into resonance with the target electronic system. As a proof of concept, we extracted the spectral distribution for the P1 electronic spin bath in diamond by using an ensemble of nitrogen-vacancy centres, and demonstrated excellent agreement with theoretical expectations. As the response of each nitrogen-vacancy spin in this experiment is dominated by a single P1 spin at a mean distance of 2.7 nm, the application of this technique to the single nitrogen-vacancy case will enable nanoscale ESR spectroscopy of atomic and molecular spin systems.
- Addresses
- School of Physics, University of Melbourne, Parkville, Victoria 3010, Australia.
- Autoren
- LT Hall
- P Kehayias
- DA Simpson
- A Jarmola
- A Stacey
- D Budker
- LCL Hollenberg
- DOI
- 10.1038/ncomms10211
- eISSN
- 2041-1723
- Externe Identifier
- PubMed Identifier: 26728001
- PubMed Central ID: PMC4728402
- Open access
- true
- ISSN
- 2041-1723
- Zeitschrift
- Nature communications
- Sprache
- eng
- Medium
- Electronic
- Online publication date
- 2016
- Open access status
- Open Access
- Paginierung
- 10211
- Datum der Veröffentlichung
- 2016
- Status
- Published
- Publisher licence
- CC BY
- Datum der Datenerfassung
- 2016
- Titel
- Detection of nanoscale electron spin resonance spectra demonstrated using nitrogen-vacancy centre probes in diamond.
- Sub types
- Research Support, Non-U.S. Gov't
- research-article
- Research Support, U.S. Gov't, Non-P.H.S.
- Journal Article
- Ausgabe der Zeitschrift
- 7
Files
https://www.nature.com/articles/ncomms10211.pdf https://europepmc.org/articles/PMC4728402?pdf=render
Datenquelle: Europe PubMed Central
- Abstract
- Electron spin resonance (ESR) describes a suite of techniques for characterizing electronic systems with applications in physics, chemistry, and biology. However, the requirement for large electron spin ensembles in conventional ESR techniques limits their spatial resolution. Here we present a method for measuring ESR spectra of nanoscale electronic environments by measuring the longitudinal relaxation time of a single-spin probe as it is systematically tuned into resonance with the target electronic system. As a proof of concept, we extracted the spectral distribution for the P1 electronic spin bath in diamond by using an ensemble of nitrogen-vacancy centres, and demonstrated excellent agreement with theoretical expectations. As the response of each nitrogen-vacancy spin in this experiment is dominated by a single P1 spin at a mean distance of 2.7 nm, the application of this technique to the single nitrogen-vacancy case will enable nanoscale ESR spectroscopy of atomic and molecular spin systems.
- Date of acceptance
- 2015
- Autoren
- LT Hall
- P Kehayias
- DA Simpson
- A Jarmola
- A Stacey
- D Budker
- LCL Hollenberg
- Autoren-URL
- https://www.ncbi.nlm.nih.gov/pubmed/26728001
- DOI
- 10.1038/ncomms10211
- eISSN
- 2041-1723
- Externe Identifier
- PubMed Central ID: PMC4728402
- Zeitschrift
- Nat Commun
- Sprache
- eng
- Country
- England
- Paginierung
- 10211
- PII
- ncomms10211
- Datum der Veröffentlichung
- 2016
- Status
- Published online
- Datum, an dem der Datensatz öffentlich gemacht wurde
- 2016
- Titel
- Detection of nanoscale electron spin resonance spectra demonstrated using nitrogen-vacancy centre probes in diamond.
- Sub types
- Journal Article
- Research Support, Non-U.S. Gov't
- Research Support, U.S. Gov't, Non-P.H.S.
- Ausgabe der Zeitschrift
- 7
Datenquelle: PubMed
- Beziehungen:
- Eigentum von